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Enhancement of coherent energy transport by disorder and temperature in light harvesting processes

หน่วยงาน Nanyang Technological University, Singapore

รายละเอียด

ชื่อเรื่อง : Enhancement of coherent energy transport by disorder and temperature in light harvesting processes
นักวิจัย : Xiong, Shi-Jie , Xiong, Ye , Zhao, Yang
คำค้น : -
หน่วยงาน : Nanyang Technological University, Singapore
ผู้ร่วมงาน : -
ปีพิมพ์ : 2555
อ้างอิง : Xiong, S. J., Xiong, Y., & Zhao, Y. (2012). Enhancement of coherent energy transport by disorder and temperature in light harvesting processes. The Journal of Chemical Physics, 137(9). , 0021-9606 , http://hdl.handle.net/10220/9400 , http://dx.doi.org/10.1063/1.4748571
ที่มา : -
ความเชี่ยวชาญ : -
ความสัมพันธ์ : The journal of chemical physics
ขอบเขตของเนื้อหา : -
บทคัดย่อ/คำอธิบาย :

We investigate the influence of static disorder and thermal excitations on excitonic energy transport in the light-harvesting apparatus of photosynthetic systems by solving the Schrödinger equation and taking into account the coherent hoppings of excitons, the rates of exciton creation and annihilation in antennas and reaction centers, and the coupling to thermally excited phonons. The antennas and reaction centers are modeled, respectively, as the sources and drains which provide the channels for creation and annihilation of excitons. Phonon modes below a maximum frequency are coupled to the excitons that are continuously created in the antennas and depleted in the reaction centers, and the phonon population in these modes obeys the Bose-Einstein distribution at a given temperature. It is found that the energy transport is not only robust against the static disorder and the thermal noise, but it can also be enhanced by increasing the randomness and temperature in most parameter regimes. Relevance of our work to the highly efficient energy transport in photosynthetic systems is discussed.

บรรณานุกรม :
Xiong, Shi-Jie , Xiong, Ye , Zhao, Yang . (2555). Enhancement of coherent energy transport by disorder and temperature in light harvesting processes.
    กรุงเทพมหานคร : Nanyang Technological University, Singapore.
Xiong, Shi-Jie , Xiong, Ye , Zhao, Yang . 2555. "Enhancement of coherent energy transport by disorder and temperature in light harvesting processes".
    กรุงเทพมหานคร : Nanyang Technological University, Singapore.
Xiong, Shi-Jie , Xiong, Ye , Zhao, Yang . "Enhancement of coherent energy transport by disorder and temperature in light harvesting processes."
    กรุงเทพมหานคร : Nanyang Technological University, Singapore, 2555. Print.
Xiong, Shi-Jie , Xiong, Ye , Zhao, Yang . Enhancement of coherent energy transport by disorder and temperature in light harvesting processes. กรุงเทพมหานคร : Nanyang Technological University, Singapore; 2555.