Thesis (M.Sc.)--Chulalongkorn University, 2015

Uranium ore can be easily detected due to various gamma-ray energies emitted from uranium daughters particularly from 238U daughters such as 214Bi, 214Pb and 226Ra. After uranium is extracted from uranium ore, only low energy gamma-rays emitted from 235U may be detected if the detector is placed in close contact to the specimen. In this research, identification and characterization of uranium bearing materials is experimentally investigated using direct measurement of gamma-rays from 235U in combination with the x-ray fluorescence (XRF) technique. Measurement of gamma-rays can be conducted by using high purity germanium (HPGe) detector or cadmium telluride (CdTe) detector while a 57Co radioisotope-excited XRF spectrometer using CdTe detector is used for elemental analysis. The proposed technique was tested with various uranium bearing specimens containing natural, depleted and enriched uranium in both metallic and powder forms. The results indicated that combination of the two techniques can be used to identify and to characterize suspicious nuclear materials not only uranium bearing materials but also Plutonium (Pu) and Thorium (Th).