In the last 25 years, piezoelectric ceramic-polymer composites have been conceptualized, prototyped, fabricated, and implemented in an array of applications encompassing medical imaging and military missions, among others. A detailed snapshot of the materials used, and a detailed account of the major innovative methods developed in making various piezoelectric ceramic-polymer composites are presented. The salient aspects of processing of such composites are summarized, and structure-processing-property relations are described using connectivity as the unifying central concept. Computer-aided design (CAD)-based fabrication methods, which result in composites whose structural complexity surpass that of composites obtained with traditional methods, are described to introduce the reader to novel concepts in processing of piezocomposites. A brief survey of some recent advances made in modeling of (0-3), (1-3), and (2-2) composites also is provided.